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Nonlinear optical response of a two-dimensional atomic crystal

2015/10/31 by Michele Merano · 2 citations
Physics and Astronomy · #Crystal (programming language) #Harmonic #High harmonic generation #Nonlinear Photonic Systems #Nonlinear optics #Nonlinear system #Photorefractive and Nonlinear Optics #Planar #Quantum Mechanics and Non-Hermitian Physics #Reflection (computer programming) #Second-harmonic generation #Surface second harmonic generation #cond-mat.mes-hall #physics.optics

paper · pdf · doi:10.1364/ol.41.000187

arxiv created 2015/12/15 · openalex publication_date 2015/12/21 · arxiv updated 2016/01/20 · openalex created_date 2016/06/24 · openalex updated_date 2026/08/05

Abstract

The theory of Bloembergen and Pershan for the light waves at the boundary of nonlinear media is extended to a nonlinear two-dimensional (2D) atomic crystal, i.e., a single planar atomic lattice, placed between linear bulk media. The crystal is treated as a zero-thickness interface, a real 2D system. Harmonic waves emanate from it. Generalization of the laws of reflection and refraction give the direction and the intensity of the harmonic waves. As a particular case that contains all the essential physical features, second-order harmonic generation is considered. The theory, due to its simplicity that stems from the special character of a single planar atomic lattice, is able to elucidate and explain the rich experimental details of harmonic generation from a 2D atomic crystal.

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