2001/08/28 by Daw-Wei Wang, S. Das Sarma · 4 citations
Materials Science · Physics and Astronomy · #Gold and Silver Nanoparticles Synthesis and Applications #Random lasers and scattering media #Theoretical and Computational Physics #cond-mat.str-el
paper · pdf · doi:10.1103/physrevb.65.125322
published as Phys. Rev. B 65, 125322 (2002).
arxiv created 2001/08/28 · openalex publication_date 2002/03/13 · arxiv updated 2009/11/30 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28
We develop a generic theory for resonant inelastic light (Raman) scattering by a conduction-band quantum plasma, taking into account the presence of a filled valence band in doped semiconductor nanostructures within a generalized resonant random-phase approximation (RPA). Our generalized RPA theory explicitly incorporates the two-step resonance process where an electron from the filled valence band is first excited by the incident photon into the conduction band before an electron from the conduction band falls back into the valence band emitting the scattered photon. We show that when the incident photon energy is close to a resonance energy, i.e., the valence-to-conduction-band gap of the semiconductor structure, the Raman-scattering spectral weight at single-particle excitation energies may be substantially enhanced even for long-wavelength excitations, and may become comparable to the spectral weight of collective charge-density excitations (plasmon). Away from resonance, i.e., when the incident photon energy is different from the band-gap energy, plasmons dominate the Raman-scattering spectrum. We find no qualitative difference in the resonance effects on the Raman-scattering spectra among systems of different dimensionalities (one, two, and three) within RPA. This is explained by the decoherence effect of the resonant interband transition on the collective motion of conduction-band electrons. Our theoretical calculations agree well (qualitatively and semiquantitatively) with the available experimental results, in contrast to the standard nonresonant RPA theory, which predicts a vanishing long-wavelength Raman spectral weight for single-particle excitations.