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Long-lived electron spin coherence in Ga-doped ZnO at room temperature

2021/03/02 by Zhen Wu, Meizhen Jiang, Jiaxing Guo +6
Physics and Astronomy · #Atomic physics #Coherence (philosophical gambling strategy) #Condensed matter physics #Dephasing #Doping #Electron #Exchange interaction #Faraday effect #Ferromagnetism #Hyperfine structure #Magnetic field #Magnetic properties of thin films #Physics #Quantum and electron transport phenomena #Quantum optics and atomic interactions #Spin (aerodynamics) #Spin polarization #physics.chem-ph #physics.optics

paper · pdf · doi:10.1103/physrevb.103.l140411

published as Phys. Rev. B 103, 140411 (2021)

arxiv created 2021/03/02 · openalex created_date 2021/03/15 · openalex publication_date 2021/04/29 · arxiv updated 2021/05/05 · openalex updated_date 2026/08/05

Abstract

Electron spin dynamics are studied in Ga-doped ZnO single crystals by time-resolved Faraday and Kerr rotation spectroscopies. Long-lived spin coherence with two dephasing processes is discovered where the characteristic time is up to 5.2 ns at room temperature. Through the dependence measurements of laser wavelength and temperature, the room-temperature long-lived spin signal is attributed to localized electrons. The spin dephasing (relaxation) processes are independent of transverse (longitudinal) magnetic fields, indicating the spin dephasing not resulting from the g-factor inhomogeneity and electron-nuclear hyperfine interaction. Phonon-induced spin dephasing/relaxation mechanism is also excluded by the magnetic field and temperature dependence measurements. It reveals that the two spin dephasing processes originate from two types of localized electrons, both of which are dominated by the anisotropic exchange Dzyaloshinskii-Moriya interaction between adjacent localized electrons.

Citations