2018/11/30 by Nikolai Christian Passler, Ilya Razdolski, I. Razdolski +6
Physics and Astronomy · #Advanced Fiber Laser Technologies #Crystal (programming language) #Dielectric #Field (mathematics) #Nanophotonics #Nonlinear Photonic Systems #Nonlinear optics #Phonon #Photorefractive and Nonlinear Optics #Polar #Polariton #Second-harmonic generation #Surface second harmonic generation #physics.optics
paper · pdf · doi:10.1021/acsphotonics.9b00290
openalex publication_date 2019/06/03 · arxiv created 2019/06/06 · arxiv updated 2019/06/07 · openalex created_date 2019/06/14 · openalex updated_date 2026/08/05
High Resolution Image Download MS PowerPoint Slide Immense optical field enhancement was predicted to occur for the Berreman mode in ultrathin films at frequencies in the vicinity of epsilon-near-zero (ENZ). Here, we report the first experimental proof of this prediction in the mid-infrared by probing the resonantly enhanced second harmonic generation (SHG) at the longitudinal optic phonon frequency from a deeply subwavelength-thin aluminum nitride (AlN) film. Employing a transfer matrix formalism, we show that the field enhancement is completely localized inside the AlN layer, revealing that the observed SHG signal of the Berreman mode is solely generated in the AlN film. Our results demonstrate that ENZ Berreman modes in intrinsically low-loss polar dielectric crystals constitute a promising platform for nonlinear nanophotonic applications.