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X-ray Rietveld refinement using Debye–Scherrer geometry

1983/10/01 by Paul Thompson, P. Thompson, I. G. Wood
Materials Science · Physics and Astronomy · #X-ray Diffraction in Crystallography #Crystallography and Radiation Phenomena #X-ray Spectroscopy and Fluorescence Analysis

paper · doi:10.1107/s0021889883010845

Abstract

A procedure for Rietveld refinement from Debye–Scherrer X-ray diffraction patterns is described, in which the effects of instrumental aberrations on the peak shapes and positions are calculated and incorporated into the refinement model. These aberrations, neglected in previous Rietveld refinement programs, can produce severe systematic errors in both the structural and non-structural parameters derived. Results presented from four materials (SiO2, AlPO4, Al2O3, LiTaO3) are in good agreement with single-crystal values and are an improvement over those previously obtained by X-ray powder diffraction.

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