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Controlling Quantum Transport through a Single Molecule

2005/08/18 by David Cardamone, D. M. Cardamone, Charles Stafford +2 · 1 citation
Computer Science · Engineering · Physics and Astronomy · #Molecular Junctions and Nanostructures #Quantum and electron transport phenomena #Quantum-Dot Cellular Automata #cond-mat.mes-hall

paper · pdf · doi:10.1021/nl0608442

published as Nano Letters 6, 2422 (2006) · 4 pages, 5 figures

arxiv created 2005/08/18 · openalex publication_date 2006/08/26 · arxiv updated 2009/12/01 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We investigate multiterminal quantum transport through single monocyclic aromatic annulene molecules, and their derivatives, using the nonequilibrium Green function approach within the self-consistent Hartree-Fock approximation. We propose a new device concept, the quantum interference effect transistor, that exploits perfect destructive interference stemming from molecular symmetry and controls current flow by introducing decoherence and/or elastic scattering that break the symmetry. This approach overcomes the fundamental problems of power dissipation and environmental sensitivity that beset nanoscale device proposals.

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