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Search for Axionlike Dark Matter Using Liquid-State Nuclear Magnetic Resonance

2025/04/22 by Walter, Julian, Maliaka, Olympia, Zhang, Yuzhe +13 · 4 citations
#Atomic Physics (physics.atom-ph) #FOS: Physical sciences #High Energy Physics - Experiment (hep-ex)

paper · doi:10.48550/arxiv.2504.16044

Abstract

We search for dark matter in the form of axionlike particles (ALPs) in the mass range 5.576741 neV/c2 - 5.577733 neV/c2 by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHz resulted in a sensitivity to the ALP-proton coupling constant of gap ≈ 3 × 10-2 GeV-1. This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment's capabilities. CASPEr-Gradient Low-Field will probe the mass range from 4.1 \peV/c2 to 17 \neV/c2 with hyperpolarized samples to boost the sensitivity beyond the astronomical limits.

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