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Spontaneous Raman scattering from metastable states of Ba+

2025/05/28 by Timothy Burke, Burke, Timothy J., Xiaoyang Shi +7
Computer Science · Physics and Astronomy · #Atomic Physics (physics.atom-ph) #FOS: Physical sciences #Quantum Computing Algorithms and Architecture #Quantum Information and Cryptography #Quantum Physics (quant-ph) #Quantum optics and atomic interactions

paper · pdf · doi:10.48550/arxiv.2505.22466

openalex publication_date 2025/05/28 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

Quantum logic gates performed via two-photon stimulated-Raman transitions in ions and atoms are fundamentally limited by spontaneous scattering errors. Recent theoretical treatment of these scattering processes has predicted no lower bound on the error rate of such gates when implemented with far-detuned lasers, while also providing an extension to metastable qubits. To validate this theoretical model, we provide experimental measurements of Raman scattering rates due to near-, and far-detuned lasers for initial states in the metastable D5/2 level of 137Ba+. The measured spontaneous Raman scattering rate is consistent with the theoretical prediction and suggests that metastable-level two-qubit gates with an error rate ≈10-4 are possible with laser excitation detuned by tens of terahertz or more.

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