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Rydberg excitons in Cu2O at millikelvin temperatures

2025/10/30 by Julian Heckötter, David Maximilian Janas, Heckötter, Julian +5
Materials Science · Physics and Astronomy · #Copper-based nanomaterials and applications #FOS: Physical sciences #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Physics of Superconductivity and Magnetism #Theoretical and Computational Physics

paper · pdf · doi:10.48550/arxiv.2510.26966

openalex publication_date 2025/10/30 · openalex created_date 2025/11/05 · openalex updated_date 2026/07/28

Abstract

Rydberg excitons in the semiconductor Cu2O have been observed in absorption experiments up to a principal quantum number of n = 28 at millikelvin temperatures [1]. Here, we extend the experimental parameter space by variing both temperature and excitation power. In particular, we show that the P excitons close to the band gap react more sensitively to an increase of the excitation power than states of the associated D exciton multiplet, even though the latter are located at comparatively higher energy. This finding is similar to the one observed when applying an external electric field, suggesting that the observed behavior arises from internal electric fields created by charged impurities that are optically ionized. At laser intensities below 1 μW/cm2, absorption lines of excitons with n=29 are observed.

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