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Optical alignment and orientation of excitons in ensemble of core/shell CdSe/CdS colloidal nanoplatelets

2022/12/12 by O. O. Smirnova, Smirnova, O. O., Ina V. Kalitukha +23
Engineering · Materials Science · Physics and Astronomy · #Chalcogenide Semiconductor Thin Films #FOS: Physical sciences #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Photonic Crystals and Applications #Quantum Dots Synthesis And Properties

paper · pdf · doi:10.48550/arxiv.2212.06134

openalex publication_date 2022/12/12 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We report on the experimental and theoretical studies of optical alignment and optical orientation effects in an ensemble of core/shell CdSe/CdS colloidal nanoplatelets. The dependences of three Stokes parameters on the magnetic field applied in the Faraday geometry are measured under continuous wave resonant excitation of the exciton photoluminescence. Theoretical model is developed to take into account both bright and dark exciton states in the case of strong electron and hole exchange interaction and random in-plane orientation of the nanoplatelets in ensemble. The data analysis allows us to estimate the time and energy parameters of the bright and dark excitons. The optical alignment effect enables identification of the exciton and trion contributions to the photoluminescence spectrum even in the absence of a clear spectral line resolution.

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