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Controlled multi-photon subtraction with cascaded Rydberg superatoms as single-photon absorbers

2021/03/29 by Nina Stiesdal, Hannes Busche, Kevin Kleinbeck +4
Computer Science · Physics and Astronomy · #Atomic physics #Cold Atom Physics and Bose-Einstein Condensates #Fine structure #Ionization #Optics #Optoelectronics #Photon #Physics #Quantum Information and Cryptography #Quantum dot #Quantum mechanics #Quantum optics and atomic interactions #Rydberg formula #Two-photon excitation microscopy #physics.atom-ph #quant-ph

paper · pdf · doi:10.1038/s41467-021-24522-w

arxiv created 2021/03/29 · openalex publication_date 2021/07/15 · arxiv updated 2021/08/04 · openalex created_date 2025/10/10 · openalex updated_date 2026/08/05

Abstract

The preparation of light pulses with well-defined quantum properties requires precise control at the individual photon level. Here, we demonstrate exact and controlled multi-photon subtraction from incoming light pulses. We employ a cascaded system of tightly confined cold atom ensembles with strong, collectively enhanced coupling of photons to Rydberg states. The excitation blockade resulting from interactions between Rydberg atoms limits photon absorption to one per ensemble and rapid dephasing of the collective excitation suppresses stimulated re-emission of the photon. We experimentally demonstrate subtraction with up to three absorbers. Furthermore, we present a thorough theoretical analysis of our scheme where we identify weak Raman decay of the long-lived Rydberg state as the main source of infidelity in the subtracted photon number and investigate the performance of the multi-photon subtractor for increasing absorber numbers in the presence of Raman decay.

Citations