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Split superconducting and time-reversal symmetry-breaking transitions, and magnetic order in Sr2RuO4 under uniaxial stress

2020/01/31 by Vadim Grinenko, Shreenanda Ghosh, Rajib Sarkar +17 · 1 citation
Physics and Astronomy · #cond-mat.supr-con #cond-mat.str-el

paper · pdf · doi:10.1038/s41567-021-01182-7

published as Nat. Phys. (2021) · 28 pages, 12 figures

arxiv created 2020/02/06 · arxiv updated 2021/03/08

Abstract

Among unconventional superconductors, Sr2RuO4 has become a benchmark for experimentation and theoretical analysis because its normal-state electronic structure is known with exceptional precision, and because of experimental evidence that its superconductivity has, very unusually, a spontaneous angular momentum, i.e. a chiral state. This hypothesis of chirality is however difficult to reconcile with recent evidence on the spin part of the order parameter. Measurements under uniaxial stress offer an ideal way to test for chirality, because under uniaxial stress the superconducting and chiral transitions are predicted to split, allowing the empirical signatures of each to be identified separately. Here, we report zerofield muon spin relaxation (ZF-μSR) measurements on crystals placed under uniaxial stresses of up to 1.05 GPa. We report a clear stress-induced splitting between the onset temperatures of superconductivity and time-reversal symmetry breaking, consistent with qualitative expectations for chiral superconductivity. We also report the appearance of unexpected bulk magnetic order under a uniaxial stress of ~ 1.0 GPa in clean Sr2RuO4.

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