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Vibrational Origin of Exchange Splitting and Chirality Induced Spin Selectivity

2020/05/14 by J. Fransson · 1 citation
Physics and Astronomy · #cond-mat.mes-hall #cond-mat.str-el

paper · pdf · doi:10.1103/physrevb.102.235416

published as Phys. Rev. B 102, 235416 (2020) · Six pages, one figure -- submitted

arxiv created 2020/05/14 · arxiv updated 2021/01/04

Abstract

Electron exchange and correlations emerging from the coupling between ionic vibrations and electrons are addressed. Spin-dependent electron-phonon coupling originates from the spin-orbit interaction, and it is shown that such electron-phonon coupling introduces exchange splitting between the spin channels in the structure. By application of these results to a model for a chiral molecular structure mounted between metallic leads, the chirality induced spin selectivity is found to become several tens of percents using experimentally feasible parameters.

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