2023/06/29 by García-Blázquez, M. A., Dednam, W., Palacios, J. J.
#Chemical Physics (physics.chem-ph) #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Mesoscale and Nanoscale Physics (cond-mat.mes-hall)
paper · doi:10.48550/arxiv.2306.17312
It is theoretically well established that a spin-dependent electron transmission generally appears in chiral systems, even without magnetic components, as long as a strong spin-orbit coupling is present in some of its elements. However, how this translates into the so-called chirality-induced spin selectivity in experiments, where the system is taken out of equilibrium, is still debated. Aided by non-equilibrium DFT-based quantum transport calculations, here we show that, when spatial symmetries that forbid a finite spin polarization in equilibrium are broken, a net spin accumulation appears at finite bias in an arbitrary two-terminal nanojunction. Furthermore, when a suitably magnetized detector is introduced in the system, the net spin accumulation, in turn, translates into a finite magneto-conductance. The symmetry prerequisites are mostly analogous to those for the spin polarization at any bias, with the vectorial nature given by the direction of magnetization.