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Polymer-encapsulated organic nanocrystals for single photon emission

2020/05/05 by Ross C. Schofield, Dominika P. Bogusz, Rowan A. Hoggarth +3
Engineering · Materials Science · Physics and Astronomy · #Anthracene #Atomic layer deposition #Fabrication #Luminescence and Fluorescent Materials #Nanocapsules #Nanocrystal #Nanophotonics #Nonlinear Optical Materials Studies #Organic Electronics and Photovoltaics #Sublimation (psychology) #Thin film #Titanium #cond-mat.mes-hall #physics.optics #quant-ph

paper · pdf · doi:10.1364/ome.396942

published as Opt. Mater. Express 10, 1586-1596 (2020) · 8 pages, comments welcome

arxiv created 2020/05/05 · openalex created_date 2020/05/13 · openalex publication_date 2020/06/04 · arxiv updated 2020/06/15 · openalex updated_date 2026/08/05

Abstract

We demonstrate an emulsion-polymerisation technique to embed dibenzoterrylene-doped anthracene nanocrystals in polymethyl methacrylate (PMMA) nanocapsules. The nanocapsules require no further protection after fabrication and are resistant to sublimation compared to unprotected anthracene. The room temperature emission from single dibenzoterrylene molecules is stable and when cooled to cryogenic temperatures we see no change in their excellent optical properties compared to existing growth methods. We also show emission from nanocapsules embedded in a thin layer of titanium dioxide, highlighting their potential for integration into hybrid nanophotonic devices.

Citations