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Colossal infrared and terahertz magneto-optical activity in a two-dimensional Dirac material

2019/05/17 by Ievgeniia O. Nedoliuk, Sheng Hu, Andre K. Geim +1 · 2 citations
Physics and Astronomy · #cond-mat.str-el #cond-mat.mes-hall

paper · pdf · doi:10.1038/s41565-019-0489-8

published as Nature Nanotechnology (2019) · 14 pages, 4 figures

arxiv created 2019/05/17 · arxiv updated 2019/07/15

Abstract

When two-dimensional electron gases (2DEGs) are exposed to magnetic field, they resonantly absorb electromagnetic radiation via electronic transitions between Landau levels (LLs). In 2DEGs with a Dirac spectrum, such as graphene, theory predicts an exceptionally high infrared magneto-absorption, even at zero doping. However, the measured LL magneto-optical effects in graphene have been much weaker than expected because of imperfections in the samples available so far for such experiments. Here we measure magneto-transmission and Faraday rotation in high-mobility encapsulated monolayer graphene using a custom designed setup for magneto-infrared microspectroscopy. Our results show a strongly enhanced magneto-optical activity in the infrared and terahertz ranges characterized by a maximum allowed (50%) absorption of light, a 100% magnetic circular dichroism as well as a record high Faraday rotation. Considering that sizeable effects have been already observed at routinely achievable magnetic fields, our findings demonstrate a new potential of magnetic tuning in 2D Dirac materials for long-wavelength optoelectronics and plasmonics.

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