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Observation of new magnetic ground state in frustrated quantum antiferromagnet spin-liquid system Cs2CuCl4

2017/08/01 by Hyeong-Jin Kim, C. R. S. Haines, Charles R. S. Haines +9 · 1 citation
Engineering · Physics and Astronomy · #Advanced Condensed Matter Physics #Antiferromagnetism #Atomic physics #Condensed matter physics #Electron #Ground state #Hydrostatic pressure #Materials science #Metastability #Perovskite Materials and Applications #Phase (matter) #Phase transition #Physics #Physics of Superconductivity and Magnetism #Quantum #Quantum mechanics #Quantum phase transition #Quantum phases #Quantum spin liquid #Spin (aerodynamics) #Spin polarization #Thermodynamics #cond-mat.str-el

paper · pdf · doi:10.1063/1.5001282

published as Low Temperature Physics 43, 901 (2017) · 9 pages, 5 figures 1 table

openalex publication_date 2017/08/01 · arxiv created 2017/12/15 · arxiv updated 2017/12/18 · openalex created_date 2020/11/23 · openalex updated_date 2026/08/06

Abstract

Cs2CuCl4 is known to possess a quantum spin-liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the application of hydrostatic pressure. We measured the magnetic properties of Cs2CuCl4 following the application and release of pressure after 3 days. We observed a previously unknown ordered magnetic phase with a transition temperature of 9 K. Furthermore, the recovered sample with new magnetic ground state possesses an equivalent crystal structure to the uncompressed one with antiferromagnetic quantum spinliquid phase.

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