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Many-body large polaron optical conductivity in SrTi1-xNbxO3

2010/03/04 by J. T. Devreese, S. N. Klimin, J. L. M. van Mechelen +1 · 1 citation
Physics and Astronomy · #cond-mat.str-el #cond-mat.mtrl-sci

paper · pdf · doi:10.1103/physrevb.81.125119

published as Phys. Rev. B 81, 125119 (2010) · to appear in Phys. Rev. B

arxiv created 2010/03/04 · arxiv updated 2015/05/18

Abstract

Recent experimental data on the optical conductivity of niobium doped SrTiO3 are interpreted in terms of a gas of large polarons with effective coupling constant αeff≈2. The theoretical approach takes into account many-body effects, the electron-phonon interaction with multiple LO-phonon branches, and the degeneracy and the anisotropy of the Ti t2g conduction band. Based on the Fröhlich interaction, the many-body large-polaron theory provides an interpretation for the essential characteristics, except -- interestingly -- for the unexpectedly large intensity of a peak at ∼130 meV, of the observed optical conductivity spectra of SrTi1-xNbxO3 without any adjustment of material parameters.

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