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Thermal conductivity ofIPA-CuCl<mml:mrow/>3: Evidence for ballistic magnon transport and the limited applicability of the Bose-Einstein condensation model

2015/04/07 by Z. Y. Zhao, Bin Tong, B. Tong +14
Materials Science · Physics and Astronomy · #Condensed matter physics #Electrical resistivity and conductivity #Magnetic field #Materials science #Organic and Molecular Conductors Research #Physics #Physics of Superconductivity and Magnetism #Quantum mechanics #Quantum, superfluid, helium dynamics #Spin (aerodynamics) #Thermal conductivity #Thermodynamics #cond-mat.str-el

paper · pdf · doi:10.1103/physrevb.91.134420

published as Phys. Rev. B 91, 134420 (2015) · 9 pages, 5 figures, accepted for publication in Phys. Rev. B

arxiv created 2015/04/07 · openalex publication_date 2015/04/17 · arxiv updated 2015/04/21 · openalex created_date 2016/06/24 · openalex updated_date 2026/08/05

Abstract

The heat transport of the spin-gapped material (CH3)2CHNH3CuCl3 (IPA-CuCl3), a candidate quantum magnet with Bose-Einstein condensation (BEC), is studied at ultralow temperatures and in high magnetic fields. Due to the presence of the spin gap, the zero-field thermal conductivity (\ensuremathκ) is purely phononic and shows a ballistic behavior at T&lt;1 K. When the gap is closed by magnetic field at H=Hc1, where a long-range antiferromanetic (AF) order of Cu2+ moments is developed, the magnons contribute significantly to heat transport and exhibit a ballistic T3 behavior at T&lt;600 mK. In addition, the low-T\phantom\rule4pt0ex\ensuremathκ(H) isotherms show sharp peaks at Hc1, which indicates a gap reopening in the AF state (H&gt;Hc1) and demonstrates limited applicability of the BEC model to IPA-CuCl3.

Citations