2010/04/06 by M. Bendele, S. Weyeneth, R. Puźniak +12 · 2 citations
Business, Management and Accounting · Chemistry · Materials Science · Physics and Astronomy · #Chemistry #Condensed matter physics #Corporate Taxation and Avoidance #Crystal structure #Crystallography #Iron-based superconductors research #Lambda #London penetration depth #Neutron diffraction #Phase (matter) #Physics #Quantum mechanics #Superconductivity #Tetragonal crystal system #cond-mat.supr-con
paper · pdf · doi:10.1103/physrevb.81.224520
published as Phys. Rev. B 81, 224520 (2010)
arxiv created 2010/04/06 · openalex publication_date 2010/06/28 · arxiv updated 2015/03/13 · openalex created_date 2016/06/24 · openalex updated_date 2026/08/05
Iron-chalcogenide single crystals with the nominal composition FeSe0.5Te0.5 and a transition temperature of Tc\ensuremath≃14.6 K were synthesized by the Bridgman method. The structural and anisotropic superconducting properties of those crystals were investigated by means of single crystal x-ray and neutron powder diffraction, superconducting quantum interference device and torque magnetometry, and muon-spin rotation (\ensuremathμSR). Room temperature neutron powder diffraction reveals that 95% of the crystal volume is of the same tetragonal structure as PbO. The structure refinement yields a stoichiometry of Fe1.045Se0.406Te0.594. Additionally, a minor hexagonal Fe7Se8 impurity phase was identified. The magnetic penetration depth \ensuremathλ at zero temperature obtained by means of \ensuremathμSR was found to be \ensuremathλab(0)=491(8) nm in the ab plane and \ensuremathλc(0)=1320(14) nm along the c axis. The zero-temperature value of the superfluid density \ensuremathρs(0)\ensuremath∝\ensuremathλ^\ensuremath-2(0) obeys the empirical Uemura relation observed for various unconventional superconductors, including cuprates and iron pnictides. The temperature dependences of both \ensuremathλab and \ensuremathλc are well described by a two-gap s+s-wave model with the zero-temperature gap values of \ensuremathΔS(0)=0.51(3) meV and \ensuremathΔL(0)=2.61(9) meV for the small and the large gap, respectively. The magnetic penetration depth anisotropy parameter \ensuremathγ_\ensuremathλ(T)=\ensuremathλc(T)/\ensuremathλab(T) increases with decreasing temperature, in agreement with \ensuremathγ_\ensuremathλ(T) observed in the iron-pnictide superconductors.