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Kapellasite: a kagome quantum spin liquid

2012/03/31 by B. Fåk, E. Kermarrec, L. Messio +11 · 2 citations
Physics and Astronomy · #cond-mat.str-el

paper · pdf

published as Phys. Rev. Lett. 109, 037208 (2012) · 5 pages, 5 figures. Published in PRL, link to supplemental materials added

arxiv created 2012/07/23 · arxiv updated 2012/07/24

Abstract

Magnetic susceptibility, NMR, muSR, and inelastic neutron scattering measurements show that kapellasite, Cu3Zn(OH)6Cl2, a geometrically frustrated spin-1/2 kagome antiferromagnet polymorphous with the herbertsmithite mineral, is a gapless spin liquid with frustrated interactions showing unusual dynamic short-range correlations of non-coplanar cuboc2 type which persist down to 20 mK. The Hamiltonian is determined from a fit of a high-temperature series expansion to thermodynamical data. The experimental data are compared to theoretical calculations using the Schwinger-boson approach.

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