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High-temperature weak ferromagnetism on the verge of a metallic state: Impact of dilute Sr doping onBaIrO3

2003/11/18 by G. Cao, Gang Cao, X. N. Lin +4 · 1 citation
Materials Science · Physics and Astronomy · #Advanced Condensed Matter Physics #Magnetic and transport properties of perovskites and related materials #Physics of Superconductivity and Magnetism #cond-mat.str-el

paper · pdf · doi:10.1103/physrevb.69.174418

arxiv created 2003/11/18 · openalex publication_date 2004/05/20 · arxiv updated 2009/12/01 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

The 5d-electron-based BaIrO3 is a nonmetallic weak ferromagnet with a Curie temperature at TC=175K. Its greatly extended orbitals generate strong electron-lattice coupling, and the magnetism and electronic structure are thus critically linked to the lattice degree of freedom. Here we report results of our transport and magnetic study on slightly Sr-doped BaIrO3. It is found that dilute Sr doping drastically suppresses TC, and instantaneously leads to a nonmetal-metal transition at high temperatures. All results highlight the instability of the ground state and the subtle relation between magnetic ordering and electron mobility. It is clear that BaIrO3 along with very few other systems represents a class of materials where the magnetic and transport properties can effectively be tuned by slight alterations in lattice parameters.

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