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Orbitally driven spin pairing in the three-dimensional nonmagnetic Mott insulatorBaVS3:Evidence from single-crystal studies

1999/11/30 by G. Mihaly, G. Mihály, I. Kézsmárki +10 · 3 citations
Materials Science · Physics and Astronomy · #Advanced Condensed Matter Physics #Anisotropy #Condensed matter physics #Electronic and Structural Properties of Oxides #Magnetic and transport properties of perovskites and related materials #Mott insulator #Pairing #Physics #Quantum mechanics #Superconductivity #cond-mat.mtrl-sci #cond-mat.str-el

paper · pdf · doi:10.1103/physrevb.61.r7831

published as Phys. Rev. B 61, R7831 (2000) · 4 pages, 5 figures, revtex, epsf, and multicol style. Problem with figures fixed. To appear in Phys. Rev. B Rap. Comm

arxiv created 2000/01/28 · openalex publication_date 2000/03/15 · arxiv updated 2009/11/30 · openalex created_date 2016/06/24 · openalex updated_date 2026/08/05

Abstract

Static electrical and magnetic properties of single crystal BaVS3 were measured over the structural (TS=240K), metal insulator (TMI=69K), and suspected orbital ordering (TX=30K) transitions. The resistivity is almost isotropic both in the metallic and insulating states. An anomaly in the magnetic anisotropy at TX signals a phase transition to an ordered low-T state. The results are interpreted in terms of orbital ordering and spin pairing within the lowest crystal-field quasidoublet. The disordered insulator at TX<T<TMI is described as a classical liquid of nonmagnetic pairs.

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