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Single-molecule spectroscopy near structured dielectrics

1998/10/06 by Carsten Henkel, Vahid Sandoghdar · 4 citations
Engineering · Materials Science · Physics and Astronomy · #Near-Field Optical Microscopy #Photonic Crystals and Applications #Quantum Dots Synthesis And Properties #physics.atom-ph #physics.optics

paper · pdf · doi:10.1016/s0030-4018(98)00519-7

published as Optics Comm. 158 (1998) 250-262 · to be published in Optics Communications (16 pages, 14 PostScript figures, uses LaTeX packages amsfonts, a4, graphicx, multicol)

arxiv created 1998/10/06 · openalex publication_date 1998/12/01 · arxiv updated 2009/12/01 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We present an analytical approach to the calculation of the linewidth and lineshift of an atom or molecule in the near field of a structured dielectric surface. For soft surface corrugations with amplitude lambda/50, we find variations of the linewidth in the ten percent region. More strikingly, the shift of the molecular resonance can reach several natural linewidths. We demonstrate that the lateral resolution is of the order of the molecule-surface distance. We give a semiquantitative explanation of the outcome of our calculations that is based on simple intuitive models.

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