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Anisotropy, Itineracy, and Magnetic Frustration in High-TCIron Pnictides

2008/11/30 by Myung Joon Han, Quan Yin, Warren E. Pickett +1 · 1 citation
Materials Science · Physics and Astronomy · #Iron-based superconductors research #Physics of Superconductivity and Magnetism #Rare-earth and actinide compounds #cond-mat.mtrl-sci #cond-mat.supr-con

paper · pdf · doi:10.1103/physrevlett.102.107003

published as Phys. Rev. Lett. 102, 107003 (2009) · Fig.4 updated: Phys. Rev. Lett (in press)

arxiv created 2009/03/09 · openalex publication_date 2009/03/11 · arxiv updated 2009/12/01 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

Using first-principles density functional theory calculations combined with insight from a tight-binding representation, dynamical mean field theory, and linear response theory, we have extensively investigated the electronic structures and magnetic interactions of nine ferropnictides representing three different structural classes. The calculated magnetic interactions are found to be short range, and the nearest (J1a) and next-nearest (J2) exchange constants follow the universal trend of J1a/2J2 approximately 1, despite their itinerant origin and extreme sensitivity to the z position of As. These results bear on the discussion of itineracy versus magnetic frustration as the key factor in stabilizing the superconducting ground state. The calculated spin-wave dispersions show strong magnetic anisotropy in the Fe plane, in contrast with cuprates.

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