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Structural Aspects of Metamagnetism inCa2−xSrxRuO4: Evidence for Field Tuning of Orbital Occupation

2004/08/01 by M. Kriener, P. Steffens, J. Baier +16 · 1 citation
Materials Science · Physics and Astronomy · #Advanced Condensed Matter Physics #Magnetic and transport properties of perovskites and related materials #Physics of Superconductivity and Magnetism #cond-mat.str-el

paper · pdf · doi:10.1103/physrevlett.95.267403

published as Phys. Rev. Lett. 95, 267403 (2005) · 4 pages, 4 figures, submitted to Physical Review Letters

arxiv created 2004/08/01 · openalex publication_date 2005/12/20 · arxiv updated 2009/12/01 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

The crystal structure of Ca(2-x)Sr(x)RuO(4) with 0.2 < or = x < or = 1.0 has been studied by diffraction techniques and by high resolution capacitance dilatometry as a function of temperature and magnetic field. Upon cooling in zero magnetic field, the crystal structure and the octahedra shrink along the c direction and elongate in the a and b planes, whereas the opposite occurs upon cooling at high field (x = 0.2 and 0.5). These findings yield evidence for an orbital rearrangement driven by temperature and magnetic field, which accompanies the metamagnetic transition at low temperature. The temperature and magnetic-field dependencies are found to be governed by the same energy scale.

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