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Mott Transition from a Spin Liquid to a Fermi Liquid in the Spin-Frustrated Organic Conductorκ−(ET)2Cu2(CN)3

2005/04/30 by Y. Kurosaki, Yasuhiro Shimizu, Y. Shimizu +5 · 8 citations
Materials Science · Physics and Astronomy · #Advanced Condensed Matter Physics #Organic and Molecular Conductors Research #Physics of Superconductivity and Magnetism #cond-mat.str-el #cond-mat.supr-con

paper · pdf · doi:10.1103/physrevlett.95.177001

published as Phys. Rev. Lett. 95, 177001 (2005) · 4 pages, 5 figures

openalex publication_date 2005/10/18 · arxiv created 2005/10/19 · arxiv updated 2009/12/01 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

The pressure-temperature phase diagram of the organic Mott insulator kappa-(ET)2Cu2(CN)3, a model system of the spin liquid on triangular lattice, has been investigated by 1H NMR and resistivity measurements. The spin-liquid phase is persistent before the Mott transition to the metal or superconducting phase under pressure. At the Mott transition, the spin fluctuations are rapidly suppressed and the Fermi-liquid features are observed in the temperature dependence of the spin-lattice relaxation rate and resistivity. The characteristic curvature of the Mott boundary in the phase diagram highlights a crucial effect of the spin frustration on the Mott transition.

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