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Low Catalyst Loadings in Olefin Metathesis: Synthesis of Nitrogen Heterocycles by Ring-Closing Metathesis

2010/02/08 by Kevin M. Kuhn, T.M. Champagne, Soon Hyeok Hong +6 · 1 citation
Chemistry · Biochemistry, Genetics and Molecular Biology · Engineering · #Synthetic Organic Chemistry Methods #Chemical Synthesis and Analysis #Fuel Cells and Related Materials

paper · doi:10.1021/ol9029808

openalex publication_date 2010/02/08 · openalex created_date 2025/10/10 · openalex updated_date 2026/08/01

Abstract

A series of ruthenium catalysts have been screened under ring-closing metathesis (RCM) conditions to produce five-, six-, and seven-membered carbamate-protected cyclic amines. Many of these catalysts demonstrated excellent RCM activity and yields with as low as 500 ppm catalyst loadings. RCM of the five-membered carbamate series could be run neat, the six-membered carbamate series could be run at 1.0 M, and the seven-membered carbamate series worked best at 0.2-0.05 M.

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