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Phonon angular momentum induced by Terahertz electric field

2025/06/06 by Hong Sun, Sun, Hong, X.J. Li +2
Physics and Astronomy · #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Quantum and electron transport phenomena #Strong Light-Matter Interactions #Topological Materials and Phenomena

paper · pdf · doi:10.48550/arxiv.2506.05715

openalex publication_date 2025/06/06 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

Despite the growing interest in phonon angular momentum (AM) in recent years, current studies remain limited to a few materials due to the constraints imposed by time reversal symmetry on macroscopic phonon AM. In this work, we theoretically investigate the generation of total phonon AM through alternating terahertz electric fields in polarized materials. In contrast to previous studies on phonon AM, here the off-diagonal elements of the phonon AM operator play an essential role. According to our formula, the large AM is generated when the energy of incident electric fields matches the frequency of optical phonons at Γ point. Furthermore, a specific resonance on the imaginary part of the response coefficient, as well as periodic regulation of the phonon AM by the phase difference of the driving field, is observed. In polar material GaN, the oscillation maximum is observed as ℏ per unit cell which can be experimentally measured through orbital magnetization induced by phonon AM. Our work offers a promising approach to generate observable phonon AM in a wider range of materials, advancing both the understanding of phonon fundamental physics and potential applications in phononic devices.

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