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Experimental Demonstration of Quantum State Expansion in a Cluster of Dipolar-Coupled Nuclear Spins

2005/01/21 by Jae-Seung Lee, Jae‐Seung Lee, A. K. Khitrin
Chemistry · Physics and Astronomy · #Advanced NMR Techniques and Applications #Atomic and Subatomic Physics Research #Molecular spectroscopy and chirality #quant-ph

paper · pdf · doi:10.1103/physrevlett.94.150504

published as Physical Review Letters 94, 150504 (2005) · 9 pages, 3 figures

arxiv created 2005/01/21 · openalex publication_date 2005/04/22 · arxiv updated 2009/12/01 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

It is experimentally demonstrated that an arbitrary quantum state of a single spin 1/2, a| upward arrow+b| downward arrow, can be converted into a superposition of the two ferromagnetic states of a spin cluster: a| upward arrow upward arrow... upward arrow upward arrow+b| downward arrow downward arrow... downward arrow downward arrow. The physical system is a cluster of seven dipolar-coupled nuclear spins of single-labeled 13C-benzene molecules in a liquid-crystalline matrix. In this complex system, the pseudopure ground state and the required controlled unitary transformations have been implemented. The experimental scheme can be considered as an explicit model of quantum measurement.

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