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Theory for transport through a single magnetic molecule: EndohedralN@C60

2004/10/31 by Florian Elste, Carsten Timm · 6 citations
Engineering · Materials Science · Physics and Astronomy · #Diamond and Carbon-based Materials Research #Graphene research and applications #Molecular Junctions and Nanostructures #cond-mat.mes-hall #cond-mat.str-el

paper · pdf · doi:10.1103/physrevb.71.155403

published as Phys. Rev. B 71, 155403 (2005) · 5 pages, 4 figures, v2: version as published

openalex publication_date 2005/04/07 · arxiv created 2005/04/19 · arxiv updated 2009/12/01 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

We consider transport through a single N@C60 molecule, weakly coupled to metallic leads. Employing a density-matrix formalism we derive rate equations for the occupation probabilities of many-particle states of the molecule. We calculate the current-voltage characteristics and the differential conductance for N@C60 in a break junction. Our results reveal Coulomb-blockade behavior as well as a fine structure of the Coulomb-blockade peaks due to the exchange coupling of the C60 spin to the spin of the encapsulated nitrogen atom.

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