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Macroscopic evidence of quantum coherent oscillations of the total spin in the Mn-[ 3×3 ] molecular nanomagnet

2003/10/02 by S. Carretta, Stefano Carretta, P. Santini +6
Materials Science · Physics and Astronomy · #Lanthanide and Transition Metal Complexes #Magnetism in coordination complexes #Organic and Molecular Conductors Research #cond-mat

paper · pdf · doi:10.1140/epjb/e2003-00331-0

published as Eur. Phys. J. B 36, 169 (2003). · 10 pages latex, 6 figures

arxiv created 2003/10/02 · openalex publication_date 2003/11/01 · arxiv updated 2009/12/01 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

Molecular nanomagnets, besides promising to open new frontiers in technology, have attracted huge interest in the scientific community because they can exhibit the phenomenon known as quantum tunnelling of the magnetization, i.e. coherent fluctuations of the direction of the total spin vector. In this paper we study a different quantum phenomenon involving fluctuations of the magnitude of the total spin vector. These fluctuations are related to the mixing between states with different spin quantum number, and imply new macroscopic effects, which we theoretically investigated in the Mn-[3x3] grid.

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