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Surface Phase Transitions Induced by Electron Mediated Adatom-Adatom Interaction

2003/03/20 by Junren Shi, Biao Wu, X. C. Xie +2
Physics and Astronomy · #cond-mat.mtrl-sci

paper · pdf · doi:10.1103/physrevlett.91.076103

published as Phys. Rev. Lett. 91, 076103 (2003) · 4 pages, 5 figures

arxiv created 2003/03/20 · arxiv updated 2009/11/30

Abstract

We propose that the indirect adatom-adatom interaction mediated by the conduction electrons of a metallic surface is responsible for the √(3)× √(3)⇔ 3× 3 structural phase transitions observed in Sn/Ge (111) and Pb/Ge (111). When the indirect interaction overwhelms the local stress field imposed by the substrate registry, the system suffers a phonon instability, resulting in a structural phase transition in the adlayer. Our theory is capable of explaining all the salient features of the √(3)× √(3)⇔ 3× 3 transitions observed in Sn/Ge (111) and Pb/Ge (111), and is in principle applicable to a wide class of systems whose surfaces are metallic before the transition.

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