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Conductivity Freeze-Out in Isotopically Pure Si-28 at milli-Kelvin Temperatures

2024/04/29 by Ben T. McAllister, Zijun C. Zhao, McAllister, Ben T. +11
Engineering · Materials Science · #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Silicon and Solar Cell Technologies #Solidification and crystal growth phenomena #Thin-Film Transistor Technologies

paper · pdf · doi:10.48550/arxiv.2404.19161

openalex publication_date 2024/04/29 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

Silicon is a key semiconducting material for electrical devices and hybrid quantum systems where low temperatures and zero-spin isotopic purity can enhance quantum coherence. Electrical conductivity in Si is characterised by carrier freeze out at around 40 K allowing microwave transmission which is a key component for addressing spins efficiently in silicon quantum technologies. In this work, we report an additional sharp transition of the electrical conductivity in a Si-28 cylindrical cavity at around 1 Kelvin. This is observed by measuring microwave resonator Whispering Gallery Mode frequencies and Q factors with changing temperature and comparing these results with finite element models. We attribute this change to a transition from a relaxation mechanism-dominated to a resonant phonon-less absorption-dominated hopping conduction regime. Characterising this regime change represents a deeper understanding of a physical phenomenon in a material of high interest to the quantum technology and semiconductor device community and the impact of these results is discussed.

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