2020/03/11 by Shunsuke Murai, Murai, Shunsuke, Gabriel W. Castellanos +7 · 1 citation
Engineering · Materials Science · Physics and Astronomy · #FOS: Physical sciences #Metamaterials and Metasurfaces Applications #Optics (physics.optics) #Orbital Angular Momentum in Optics #Plasmonic and Surface Plasmon Research
paper · pdf · doi:10.48550/arxiv.2003.05076
openalex publication_date 2020/03/11 · openalex created_date 2020/03/23 · openalex updated_date 2026/07/28
We demonstrate an enhanced emission of high quantum yield molecules coupled to dielectric metasurfaces formed by periodic arrays of polycrystalline silicon nanoparticles. Radiative coupling of the nanoparticles, mediated by in-plane diffraction, leads to the formation of collective Mie scattering resonances or Mie surface lattice resonances (M-SLRs), with remarkable narrow line widths. These narrow line widths and the intrinsic electric and magnetic dipole moments of the individual Si nanoparticles allow to resolve electric and magnetic M-SLRs. Incidence angle- and polarization-dependent extinction measurements and high-accuracy surface integral simulations show unambiguously that magnetic M-SLRs arise from in- and out-of-plane magnetic dipoles, while electric M-SLRs are due to in-plane electric dipoles. Pronounced changes in the emission spectrum of the molecules are observed, with almost a 20-fold enhancement of the emission in defined directions of molecules coupled to electric M-SLRs, and a 5-fold enhancement of the emission of molecules coupled to magnetic M-SLRs. These measurements demonstrate the potential of dielectric metasurfaces for emission control and enhancement, and open new opportunities to induce asymmetric scattering and emission using collective electric and magnetic resonances.