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On-chip interference of scattering from two individual molecules in plastic

2023/01/26 by Dominik Rattenbacher, Rattenbacher, Dominik, Alexey Shkarin +9 · 1 citation
Engineering · Physics and Astronomy · #FOS: Physical sciences #Mechanical and Optical Resonators #Optics (physics.optics) #Photonic Crystals and Applications #Photonic and Optical Devices #Quantum Physics (quant-ph)

paper · pdf · doi:10.48550/arxiv.2301.11024

openalex publication_date 2023/01/26 · openalex created_date 2025/10/10 · openalex updated_date 2026/08/01

Abstract

Integrated photonic circuits offer a promising route for studying coherent cooperative effects of a controlled collection of quantum emitters. However, spectral inhomogeneities, decoherence and material incompatibilities in the solid state make this a nontrivial task. Here, we demonstrate efficient coupling of a pair of organic molecules embedded in a plastic film to a TiO2 microdisc resonator on a glass chip. Moreover, we tune the resonance frequencies of the molecules with respect to that of the microresonator by employing nanofabricated electrodes. For two molecules separated by a distance of about 8 μm and an optical phase difference of about π/2, we report on a large collective extinction of the incident light in the forward direction and the destructive interference of its scattering in the backward direction. Our work sets the ground for the coherent coupling of several molecules via a common mode and the realization of polymer-based hybrid quantum photonic circuits.

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