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Double Resonant Tunable Second Harmonic Generation in Two-dimensional Layered Materials through Band Nesting

2021/08/16 by Sudipta Biswas, Biswas, Sudipta Romen, Jin Yu +11 · 1 citation
Engineering · Physics and Astronomy · #FOS: Physical sciences #Mechanical and Optical Resonators #Optics (physics.optics) #Photonic and Optical Devices #Photorefractive and Nonlinear Optics

paper · pdf · doi:10.48550/arxiv.2108.06900

openalex publication_date 2021/08/16 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We proposed a mechanism to generate giant anisotropic second harmonic nonlinear response via double resonance effect, achieved through band nesting via electronic bandstructure engineering. The ideal band setup would be a triplet of nested bands separated by the fundamental resonance energy, ℏω. We demonstrate theoretically that the proposed phenomenon can be realized in bilayer SnS by band tuning with perpendicular electrical bias, which maximizes the second harmonic susceptibility by several orders of magnitude. Moreover, the tunability of the polarization anisotropy can be useful for realizing novel polarization-sensitive devices.

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