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Fluence dependent delay of Ni in an FeNi alloy supports an exchange based origin

2025/03/11 by Somnath Jana, Ronny Knut, Jana, Somnath +21
Earth and Planetary Sciences · Materials Science · Physics and Astronomy · #FOS: Physical sciences #Magnetic properties of thin films #Materials Science (cond-mat.mtrl-sci) #Nanoporous metals and alloys #nanoparticles nucleation surface interactions

paper · pdf · doi:10.48550/arxiv.2503.08811

openalex publication_date 2025/03/11 · openalex created_date 2025/10/13 · openalex updated_date 2026/07/28

Abstract

The delayed demagnetization in Ni relative to Fe in the ultrafast demagnetization studies in FeNi alloy has led to two competing theoretical explanations: The Inhomogeneous Magnon Generation (IMG) and the Optically Induced Spin Transfer (OISTR) model. The IMG attributes the delay to the preferential magnon generation at the Fe sites and its subsequent propagation to Ni, while OISTR proposes direct spin transfer from Ni to Fe. In this study, we employ element-resolved extreme ultraviolet spectroscopy to investigate the effect of excitation strength on this delay, aiming to resolve the controversy. The data indicate a significant reduction in the delay with increasing fluence, which is inconsistent with the theoretical predictions of OISTR. These findings, in conjunction with the observation of a saturation of Fe demagnetization at the onset of Ni demagnetization, indicate that a spin-wave instability within the IMG framework may provide a potential explanation for the experimental results.

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