2023/05/12 by Edvin Olofsson, Olofsson, Edvin, Jan Marcus Dahlström +1
Physics and Astronomy · #Laser-Matter Interactions and Applications #Spectroscopy and Quantum Chemical Studies #Atomic and Molecular Physics
paper · pdf · doi:10.48550/arxiv.2305.07363
Non-perturbative resonant multiphoton ionization (1+1) is studied using the resolvent operator technique. Scaling parameters for effective two-level Hamiltonians are computed for hydrogen and helium atoms to provide a quantitative description of Rabi oscillations at XUV wavelengths, which were recently observed using a seeded Free-Electron Laser [S. Nandi et al., Nature 608, 488-493 (2022)]. The resulting photoelectron spectra exhibit a range of Autler-Townes doublets, which are studied for different intensities, detunings and interaction times. We identify a photoelectron signature that originates from stabilization against ionization of helium atoms interacting with intense circularly polarized XUV light. Thus, our work shows how it is possible to test the prediction of dressed-atom stabilization by Beers and Armstrong [B. L. Beers and L. Armstrong, Phys. Rev. A 12, 2447 (1975)], without the demanding requirement of atomic saturation in the time domain.