2020/08/26 by Juan C. Verduzco, Verduzco, Juan C., John N. Vergados +5
Engineering · Materials Science · #Advanced Battery Materials and Technologies #Applied Physics (physics.app-ph) #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Perovskite Materials and Applications #Polyoxometalates: Synthesis and Applications
paper · pdf · doi:10.48550/arxiv.2008.11855
openalex publication_date 2020/08/26 · openalex created_date 2022/07/26 · openalex updated_date 2026/07/28
Hybrid electrolyte materials comprising polymer-ionic salt matrixes embedded\nwith garnet particles constitute a promising class of materials for the\nrealization of all-solid-state batteries. In addition to providing solutions to\nthe safety issues inherent to current liquid electrolytes, hybrid polymer\nelectrolytes offer advantages over other solid-state electrolytes. This is\nbecause their functional properties such as ionic conductivity, electrochemical\nstability, mechanical and thermal properties can be tailored to a particular\napplication by independently optimizing the properties of the constituent\nmaterials. Thereby, providing a rational approach to solving bottlenecks\ncurrently preventing solid-state electrolytes from practical implementation\ninto battery devices. This review starts with a survey of solid-state\nelectrolytes, focusing on their materials and ion transport limitations. Next,\nwe summarize the current understanding of transport mechanisms in composite\npolymer electrolytes (CPEs) with the purpose of identifying materials solutions\nfor further improving their properties. The overall goal of the review is to\nfoster heightened research interest in these hybrid structures to rapidly\nadvance development of future all-solid-state battery devices.\n