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Fingerprints of a charge ice state in the doped Mott insulator Nb3Cl8

2024/05/29 by E. A. Stepanov, Stepanov, Evgeny A.
Decision Sciences · Physics and Astronomy · #Cold Atom Physics and Bose-Einstein Condensates #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Quantum many-body systems #Strongly Correlated Electrons (cond-mat.str-el) #scientometrics and bibliometrics research

paper · pdf · doi:10.48550/arxiv.2405.19114

openalex publication_date 2024/05/29 · openalex created_date 2024/05/31 · openalex updated_date 2026/07/28

Abstract

The interplay between strong electronic correlations and the inherent frustration of certain lattice geometries is a common mechanism for the formation of nontrivial states of matter. In this work, we theoretically explore the collective electronic effects in the monolayer Nb3Cl8, a recently discovered triangular lattice Mott insulator. Our advanced many-body numerical simulations predict the emergence of a phase separation region upon doping this material. Notably, in close proximity to the phase separation, the static charge susceptibility undergoes a drastic change and reveals a distinctive bow-tie structure in momentum space. The appearance of such a fingerprint in the context of spin degrees of freedom would indicate the formation of a spin ice state. This finding allows us to associate the observed phase separation to a charge ice state, a state with a remarkable power law dependence of both the effective exchange interaction and correlations between electronic densities in real space.

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