2025/04/03 by Jun-Yong Yan, Yan, Jun-Yong, Paul C. A. Hagen +19 · 1 citation
Biochemistry, Genetics and Molecular Biology · Physics and Astronomy · #Advanced Fluorescence Microscopy Techniques #Digital Holography and Microscopy #FOS: Physical sciences #Optics (physics.optics) #Orbital Angular Momentum in Optics #Quantum Physics (quant-ph)
paper · pdf · doi:10.48550/arxiv.2504.02753
openalex publication_date 2025/04/03 · openalex created_date 2025/10/16 · openalex updated_date 2026/07/28
Quantum emitters driven by resonant two-photon excitation are a leading source for deterministically generated entangled photon pairs, essential for scalable photonic quantum technologies. However, conventional resonant schemes are highly sensitive to laser power fluctuations and pose additional experimental challenges for emitters with small biexciton binding energies. Here, we demonstrate how biexciton preparation schemes with significantly improved robustness and reduced laser filtering requirements can be identified using a novel design principle beyond resonant and adiabatic driving: ultrafast single-shot Floquet driving. This is achieved by employing two strongly and symmetrically detuned dichromatic pulses, whose superposition generates a stroboscopic Hamiltonian that enables direct coupling between ground and biexciton states. Moreover, a pulse delay serves as a tuning knob, introducing an effective magnetic field that concentrates the Bloch sphere trajectory at the biexciton state for a wide range of parameters, making biexciton preparation particularly robust. Experimentally, we achieve a biexciton occupation exceeding 96% and preserve photon-pair entanglement with a fidelity of 93.4%. Our scheme highlights the great impact of Floquet-engineered multicolour excitation protocols for on-demand quantum light sources.