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Tunable magnetocaloric effect and enhanced refrigerant capacity in composite-like oxide heterostructures

2022/11/04 by M. Abbasi Eskandari, S. Ghotb, Eskandari, Mohammad Abbasi +5
Materials Science · Physics and Astronomy · #Advanced Thermodynamics and Statistical Mechanics #Advanced Thermoelectric Materials and Devices #Applied Physics (physics.app-ph) #FOS: Physical sciences #Magnetic and transport properties of perovskites and related materials #Materials Science (cond-mat.mtrl-sci)

paper · pdf · doi:10.48550/arxiv.2211.02715

openalex publication_date 2022/11/04 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We report a detailed study of the magnetocaloric effect in heterostructures of La2NiMnO6 and La2/3Sr1/3MnO3. The shape, width and magnitude of the temperature dependence of the magnetic entropy change (ΔSm) for these multilayer samples can be tuned and controlled by changing their layout. A large ΔSm over a wide temperature range which goes beyond room temperature is observed in all samples. We observe a temperature-independent table-top-like ΔSm over a temperature range as large as 100 K in the trilayer samples. La2NiMnO6 double perovskite with multiple magnetic phase transitions is the key to tuning and shaping the temperature dependence of the magnetic entropy changes to suit the requirements of several cooling cycles.

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