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Observation of Spin Fluctuations in a High-Tc Parent Compound Using Resonant Inelastic X-ray Scattering

2008/06/27 by Byron Freelon, P. G. Medaglia, Freelon, B. +27
Materials Science · Physics and Astronomy · #Diamond and Carbon-based Materials Research #FOS: Physical sciences #Magnetic properties of thin films #Physics of Superconductivity and Magnetism #Superconductivity (cond-mat.supr-con)

paper · pdf · doi:10.48550/arxiv.0806.4432

openalex publication_date 2008/06/27 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We report the first observation of soft-x-ray scattering from spin fluctuations in a high-Tc parent compound. An antiferromagnetic charge transfer insulator, CaCuO2, was irradiated by Cu M-edge soft x-rays. Ultra-high resolution measurements of scattered intensity revealed magnon-magnon excitations, due to spin exchange scattering, as low-energy loss features. The process is analogous to optical Raman scattering. The spectra provide the first measurement of the two-magnon excitation energy and the antiferromagnetic exchange parameter in infinite-layer CaCuO2. The results reveal resonant inelastic soft x-ray scattering as a novel probe of the spin dynamics in cuprates.

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