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Strongly anisotropic magnetocaloric effect in a dipolar magnet LiGdF4

2023/07/12 by G.Iu. Andreev, I. V. Romanova, Andreev, G. Iu. +11
Materials Science · Physics and Astronomy · #Advanced Thermodynamics and Statistical Mechanics #FOS: Physical sciences #Magnetic and transport properties of perovskites and related materials #Materials Science (cond-mat.mtrl-sci) #Strongly Correlated Electrons (cond-mat.str-el) #Theoretical and Computational Physics

paper · pdf · doi:10.48550/arxiv.2307.06111

openalex publication_date 2023/07/12 · openalex created_date 2025/10/10 · openalex updated_date 2026/08/03

Abstract

We report the detailed study of the magnetocaloric effect (MCE) in a dipolar-Heisenberg magnet LiGdF4 using magnetization measurements performed on a single crystal sample. Entropy variation on isothermal demagnetization from the magnetic field up to 3 T is determined in the temperature range 2-10 K for two principal directions of the applied field (parallel and perpendicular to the tetragonal c-axis of the crystal). The MCE is found to be highly anisotropic, with the cooling efficiency being up to twice higher at H∥ c. The results are nicely interpreted in the frame of a conventional molecular field approach taking into account considerable anisotropy of the paramagnetic Curie-Weiss temperature. These results are compared to earlier studies of MCE in powder samples of LiGdF4 [T. Numazawa et al., AIP Conf. Proc. 850, 1579 (2006)] as well as with analogous data for other well known magnetocaloric materials. Our findings may open new possibilities to enhance the efficiency of magnetic refrigeration in the liquid helium-4 temperature range.

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