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First principles calculation of the phonons modes in the hexagonal \rm YMnO3 ferroelectric and paraelectric phases

2012/03/08 by Julien Varignon, S. Petit, Varignon, Julien +3
Engineering · Materials Science · #FOS: Physical sciences #Geophysics and Sensor Technology #Materials Science (cond-mat.mtrl-sci) #Multiferroics and related materials #Solid-state spectroscopy and crystallography #Strongly Correlated Electrons (cond-mat.str-el)

paper · pdf · doi:10.48550/arxiv.1203.1752

openalex publication_date 2012/03/08 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

The lattice dynamics of the \rm YMnO3 magneto-electric compound has been investigated using density functional calculations, both in the ferroelectric and the paraelectric phases. The coherence between the computed and experimental data is very good in the low temperature phase. Using group theory, modes continuity and our calculations we were able to show that the phonons modes observed by Raman scattering at 1200K are only compatible with the ferroelectric P63 cm space group, thus supporting the idea of a ferroelectric to paraelectric phase transition at higher temperature. Finally we proposed a candidate for the phonon part of the observed electro-magnon. This mode, inactive both in Raman scattering and in Infra-Red, was shown to strongly couple to the Mn-Mn magnetic interactions.

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