2025/06/04 by Glick, Jeremy, Anderson, Brielle E., Nunley, T. Nathan +4 · 1 citation
#Atomic Physics (physics.atom-ph) #FOS: Physical sciences
paper · doi:10.48550/arxiv.2506.04504
The common approach for producing Rydberg atoms in warm vapor cells is with lasers arranged in a counter-propagating, collinear configuration. Doppler effects in these configurations reduce the efficiency of excitation to the Rydberg state while also producing broadened spectral features. In this work, we demonstrate a three-laser Doppler-free excitation using laser beams whose k-vectors sum to zero, resulting in an enhancement in the Rydberg density and narrowed spectral features. A three-times enhancement to Rydberg density along with a near four-times reduction in spectroscopic line-widths are observed compared to a collinear configuration. This Doppler-free configuration could prove beneficial to Rydberg atomic technologies, such as electric field sensing with small volumes or deterministic photon sources.