2022/02/12 by Hiroshi Ôike, Oike, Hiroshi, Kazuya Miyagawa +7
Decision Sciences · Physics and Astronomy · #Advanced Condensed Matter Physics #Cold Atom Physics and Bose-Einstein Condensates #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Personal Information Management and User Behavior #Strongly Correlated Electrons (cond-mat.str-el) #Superconductivity (cond-mat.supr-con)
paper · pdf · doi:10.48550/arxiv.2202.06032
openalex publication_date 2022/02/12 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28
Quantum spin liquid states, in which spins are quantum-mechanically delocalized in direction, have been so far studied for charge-localized Mott insulators arising from strong repulsive interaction. Recently, however, it was found that the doped Mott insulator with a triangular lattice, κ-(ET)4Hg2.89Br8, exhibits both spin-liquid-like magnetism and metallic electrical conduction. Thus, it is now possible to experimentally explore how the spin liquidity affects the electrical conduction, an issue that has received a great deal of theoretical attention. Here, with a newly developed method to combine uniaxial and hydrostatic pressures, we investigate the electrical conduction in the doped Mott insulator with controlling the triangular lattice geometry and the repulsion strength which determines the spin-liquidity and Mottness, respectively. We found that, in a strongly interacting regime, the electronic state drastically changes from an insulator to a Fermi liquid via a non-Fermi liquid with varying geometrical frustration, which suggests that spin liquidity promotes delocalization of charges. This result indicates that frustration in spin degrees of freedom has a decisive impact on the transport of charges through the entanglement of spin and charge in a doped Mott insulator.