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Probing moire excitons in MoSe2/WSe2 heterobilayers by combined micro-photoluminescence and lateral force microscopy

2025/11/20 by Caussou, L., Moutaabbid, H., Bernard, M. +6
Materials Science · Physics and Astronomy · #2D Materials and Applications #FOS: Physical sciences #Force Microscopy Techniques and Applications #Mechanical and Optical Resonators #Mesoscale and Nanoscale Physics (cond-mat.mes-hall)

paper · doi:10.48550/arxiv.2511.16539

openalex publication_date 2025/11/20 · openalex created_date 2025/11/23 · openalex updated_date 2026/07/28

Abstract

We study interlayer excitons in MoSe2/WSe2 heterobilayers, by combining lateral force microscopy and micro-photoluminescence spectroscopy. This allows us to correlate the spatial profile of the moiré superlattice with the distribution of optically active states accessible to interlayer excitons. In heterostructures where a few degrees twist angle is imposed between the MoSe and WSe crystallographic axes, we show that a continuous moiré lattice is realized across areas close to the optical diffraction limit. In such regions, the photoluminescence reduces to a few narrow-band lines only, energetically distributed consistently with the geometry of the moiré lattice. This correlation reveals that interlayer excitons explore a controlled periodic confinement, paving the way towards implementations of Bose-Hubbard models.

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