2023/11/30 by Kohei Nagai, Nagai, Kohei, Takuya Okamoto +7 · 3 citations
Physics and Astronomy · Materials Science · #Orbital Angular Momentum in Optics #Mechanical and Optical Resonators #Metamaterials and Metasurfaces Applications
paper · pdf · doi:10.48550/arxiv.2311.18500
Symmetries essentially provide conservation rules in nonlinear light-matter interactions, that facilitate control and understanding of photon conversion processes or electron dynamics. Since anisotropic solids have rich symmetries, they are strong candidate to control both optical micro- and macroscale structures, namely spin (circular polarization) and orbital angular momentum (spiral wavefront), respectively. Here, we show structured high harmonic generation linked to the anisotropic symmetry of a solid. By strategically preserving a dynamical symmetry arising from the spin-orbit interaction of light, we generate multiple orbital angular momentum states in high-order harmonics. The experimental results exhibit the total angular momentum conservation rule of light even in the extreme nonlinear region, which is evidence that the mechanism originates from a dynamical symmetry. Our study provides a deeper understanding of multiscale nonlinear optical phenomena and a general guideline for using electronic structure to control structured light, such as through Floquet engineering.